Characterization and thermoluminescence behavior of beta irradiated NaBaBO3 phosphor synthesized by combustion method


Oğlakçı M., Akça S., Halefoğlu Y. Z., Doğan T., Ayvacıklı M., Karabulut Y., ...More

CERAMICS INTERNATIONAL, vol.45, pp.7011-7017, 2019 (SCI-Expanded) identifier identifier

  • Publication Type: Article / Article
  • Volume: 45
  • Publication Date: 2019
  • Doi Number: 10.1016/j.ceramint.2018.12.202
  • Journal Name: CERAMICS INTERNATIONAL
  • Journal Indexes: Science Citation Index Expanded (SCI-EXPANDED), Scopus
  • Page Numbers: pp.7011-7017
  • Keywords: NaBaBO3, XRD, SEM, Thermoluminescence, TLanal software, Peak shape method, GLOW CURVES, DECONVOLUTION
  • Çukurova University Affiliated: Yes

Abstract

NaBaBO3 host material was synthesized using the combustion method. In order to optimize the performance of the material, effects of sintering temperatures varying from 600 degrees to 1000 degrees C were investigated. The sintering temperature and dwell time were found to have pronounced effects on the pure NaBaBO3 material. X-ray powder diffraction (XRD) and scanning electron microscopy (SEM) techniques were used to confirm the phase formation and examine the surface morphology of the prepared powder material, respectively. TL behavior of NaBaBO3 was studied at various beta doses. It is seen that the sample exhibits well resolved TL glow peak at a peak temperature about 175 degrees C and corresponding TL intensity increases with the increasing beta dose. However, TL glow peak slightly shifts to lower temperature with the increasing beta dose level. This is the first TL report of a phosphor with a NaBaBO3 host. The TL kinetic parameters were estimated by the peak shape (PS) method and CGCD software. TL glow curves of NaBaBO3 consist of several traps and exhibited second order kinetics. A possible TL mechanism was also discussed using the energy level model. The obtained results can provide valuable knowledge related to the investigation of the intrinsic nature characteristics of NaBaBO3 in research fields pertaining to dosimetry.

NaBaBO3 host material was synthesized using the combustion method. In order to optimize the performance of the material, effects of sintering temperatures varying from 600 degrees to 1000 degrees C were investigated. The sintering temperature and dwell time were found to have pronounced effects on the pure NaBaBO3 material. X-ray powder diffraction (XRD) and scanning electron microscopy (SEM) techniques were used to confirm the phase formation and examine the surface morphology of the prepared powder material, respectively. TL behavior of NaBaBO3 was studied at various beta doses. It is seen that the sample exhibits well resolved TL glow peak at a peak temperature about 175 degrees C and corresponding TL intensity increases with the increasing beta dose. However, TL glow peak slightly shifts to lower temperature with the increasing beta dose level. This is the first TL report of a phosphor with a NaBaBO3 host. The TL kinetic parameters were estimated by the peak shape (PS) method and CGCD software. TL glow curves of NaBaBO3 consist of several traps and exhibited second order kinetics. A possible TL mechanism was also discussed using the energy level model. The obtained results can provide valuable knowledge related to the investigation of the intrinsic nature characteristics of NaBaBO3 in research fields pertaining to dosimetry.